Solved it. For anyone trying to accomplish this with Gravity Forms, the following is what worked for me. Your mileage may vary.
First, it's a good idea to give your form a custom css class in the GF Form Settings "Advanced" tab. Then in your stylesheet:
.gform_wrapper { max-width: 100%; }
.gform_wrapper.yourcustomclass_wrapper {
position: relative;
margin:0;
padding:0;
width: 600px;
max-width: 100%;
}